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Dodel and H. Taube, Z . phys. Chem. (Frankfurt), 1965,44, 92. J. P. Candlin, J. Halpern, and D. L. Trimm, J. Amer. Chem. ,1964, 86, 1019. F. Nordmeyer and H. Taube, J. Amer. Chem. ,1968,90, 1163. J. Doyle and A. G . Sykes, J. Chem. (A), 1968, 2836. R. G. Gaunde and H. Taube, Inorg. , 1970,9,2627. A. B. Hoffmann and H. Taube, Inorg. , 1968,7, 1971. P. K. Zia, R. B. Fisher, and W. K. Wilmarth, Abs. Amer. Chem. ,161st Meeting, Los Angeles, 1971, Inorg. 027. 023 37 38 39,4 40 41 42 43a 24 24 270 27c 27“ 29 33e 33e 33e trenen =Caminoethyl-l,4,7,1O-tetra-azadecane.
3 - AH* 58 58 58 58 58 58 58 58 58 58 58 58 57 57 57 57 57 57 57 57 57 57 Ref. 3 2 @a 3 9 4 2 0 00 N a 2 % (p-form bz) = p-formylbenzoato. * Acid-dependent pathway. Units are I* mol-a s-l. (m-form bz) = m-formylbenzoato. e Adjacent 3 attack. f Path leading to ligand release. 0 benz = benzoato. 1M. See text for formulae of tetranuclear complexes. Ic tim = quadridentate macrocycle, 2,3,9,10-tetrarnethy1-1,4,8,11-tetra-azacyclotetradeca-1,3,8,10-tetraene. 2 Reductant is [Cr(CN)a]4-. Tetranuclear complex (7); see p.
B. King, D. M. Braitsch, and P. N. S. Chem. , 1972, 1072. E. E. Mercer and L. W. Gray, J. Amer. Chem. , 1972, 94, 6426. K. B. Yatsimirskii, L. P. Tikhonova, L. N. Zakrevskaya, and I. P. Svarovskaya, Zhur. neurg. , 1972, 17, 3206. A. Nuyt and M. Zador, Canad. J. , 1972,50,2413. G. D. Watt, J. Amer. Chem. ,1972, 94, 7351. 31 Reactions Between Two Metal Complexes cerium(w) may also be important since a stable intermediate is formed when CeIY : [Ru(NH3)&02+]is < 3 . 69 The reaction is second-order overall and in 20-30% Bu,PO, the rate constant is about two orders of magnitude lower than for the corresponding aqueous reaction at the same temperature.